Is the chip used to store the key temper resistant comparable with the hardware lever of security used for smart cards?
Yes and no. The chip is a standard NFC chip so technically depending how you encode it you COULD enforce smart card level security, but it's not really necessary for most users. It's more important to use it with Multi-Sig so that if someone gets ahold of one, they still don't have your bitcoin. You could make possession of all of the devices more difficult to use, if that was really your goal, but I had created the device with the idea that once you have all the devices it's easy to get your bitcoin in safe reliable way. People are better at protecting physical goods then they are digital- hiding something someplace secure or putting it in a vault is a more reliable and intuitive way of protecting something than encrypting it in fancy ways. The casual user is more likely to mess up the encryption part, not the putting it in their safe part.